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Variation of Flux and Energy of 14 Mev Neutrons With Variation of Matrix Around A Sample

Ranjita Mandal1,2*, Anita Thanekar2, G. R. Pansare2, 3, V. N. Bhoraskar2 and D. Sengupta1

1Department of Geology and Geophysics, I.I.T., Kharagpur - 721 302, India. 

2Department of Physics, University of Poona, Pune - 411 002, India.

3H.V. Desai College, Pune - 411 002, India.

DOI : http://dx.doi.org/10.13005/msri/080223

Article Publishing History
Article Received on : 1 Oct 2011
Article Accepted on : 18 Nov 2011
Article Published :
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ABSTRACT:

Here a method has been described to study the attenuation of flux and energy of the neutrons passing through different materials. Variation of activity of the irradiated and activated sample by 14 MeV neutrons was observed by changing the matrix around it. The sample was a combination of Aluminium foil and copper powder placed at 0o position (position of maximum flux) and the matrices were Air, Water, Iron, sand and carbon powder.

KEYWORDS: Matrix; Cross-section; 14 MeV neutrons; Activation method; Neutron flux; Neutron energy

Copy the following to cite this article:

Mandal R, Thanekar A, Pansare G. R, Bhoraskar V. N, Sengupta D. Variation of Flux and Energy of 14 Mev Neutrons With Variation of Matrix Around A Sample. Mat.Sci.Res.India;8(2)


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Mandal R, Thanekar A, Pansare G. R, Bhoraskar V. N, Sengupta D. Variation of Flux and Energy of 14 Mev Neutrons With Variation of Matrix Around A Sample. Mat.Sci.Res.India;8(2). Available from: http://www.materialsciencejournal.org/?p=2686


Introduction

The 14 MeV neutron generator1 used for the present work generates neutrons of energy 14.77 MeV and has a flux of 108 n/cm2/sec. When a sample is irradiated then the induced activity 2 in the sample is

A=N σ F

Where A, N, σ and F denote activity induced in the irradiated sample, the neutron flux, cross-section of the reaction through which activity is induced and flux of the neutrons respectively.

Now, if two samples 1 and 2 are irradiated simultaneously then the activity induced will be

A1=N1σ1F  and  A2=N2σ2F

F being same for both because of simultaneous irradiation. Taking the ratio of the two activities, we get 

A1/A2=Kσ12

Where K=N1/N2 is constant for constant weights of sample 1 and 2. A1/A2 is constant when σ12 is constant. And σ12 is constant when the energy of the incident neutrons is constant. As with the variation of energy both σ1 and σ2 vary, so does the ratio σ12. So knowing this ratio the value of the energy E can be found as σ12 has a constant value for a particular value of E. The actual neutron source is surrounded by an iron water cooling jacket. The results can help to understand the attenuation of the neutron energy and flux and corresponding corrections can be made in the cross-section values obtained from the neutron activation analysis method using these neutrons.

Material and Methods

For observing the variation of flux and energy of neutrons, experiment was done by irradiating two samples simultaneously and varying the matrix around it and noting the variation of activity.

The sample and matrix used along with the concerned data is given in Table 1 and 2.

Table 1: Samples used

Table 1
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 Table 2: Matrices used

Table 2
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The excitation curves3, 4 are shown in figures 1 and 2. The samples taken together, Copper in powder form and Aluminium as foil within a polythene bag were irradiated with different matrices around it one by one. The time of irradiation, cooling and counting were 10, 2 and 10 minutes respectively. These two samples were taken because of the following reasons:

Easily available

Comparable half life5 of the products allowed to take same irradiation time, that is, around 10 minutes.

Excitation curve shows that in the energy region concerned (12-15 MeV), the slope is different (for copper it is increasing and for aluminium it is decreasing) and so σ12 varies with energy or we can say d(σ12) /dE is high and easily noticeable even for small energy change.

Figure 1: Excitation curve for the reaction Cu63(n,2n)Cu62

Figure 1
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Figure 2: Excitation curve for the reaction Al27(n,p)Mg27

Figure 2
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Results and Discussion

The ratio K of number of atoms of Copper to number of atoms of aluminium, that is, NAl/NCu has a value of 0.34. And as such the cross-section ratio is given as

σCuA l =  (0. 34)*(ACu / AAl)

Where ACu / AAl is the activity ratio of copper to aluminium.The value of sCu/sA l gives the value of energy of the neutrons.The variation of flux and energy of the neutrons with variation of matrix around the sample as obtained are shown in Table 3.

Table 3: Variation of neutron energy with matrices

Table 3
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The maximum variation of neutron flux and energy is for carbon matrix. And the least variation is for iron powder.

Acknowledgements

I am thankful to the Council of Scientific and Industrial Research and Department of Science and Technology for their financial support.

References

  1. V.N. Bhoraskar, Ind. J. Pure and Appl. Phys.,27: 648, (1989).
  2. L.F. Curtiss, An introduction to neutron physics, D. Van Nostrand Company, Inc., Princeton, New Jersey, (1959) .
  3. Technical report series no.273, Handbook on nuclear activation data by international atomic energy agency.
  4. EXFOR Nuclear Reaction Data, http:// www.nds.iaea.org/exfor
  5. C.M. Lederer, J.M. Hollander, and I. Perlman, Table of Isotopes, John Wiley and. Sons, New York (1967).
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